AbstractAn experimental investigation was conducted into establishing relationships between the processing variables and the mechanical properties of compression‐molded parts of sheet molding compounds (SMC). Emphasis was placed on investigating the effects on the tensile properties, impact strength, and dynamic mechanical properties of composite specimens, of low‐profile additives, and of treating glass fibers (for reinforcement) with sizing chemicals. The processing variables investigated were cure time, mold temperature, and mold pressure. It was found that: (1) An optimum cure time and mold temperature exist for achieving molded SMC composites of the greatest tensile and impact strengths; (2) Of the four different types of low‐profile thermoplastic additives employed, the poly(vinyl acetate) modified with acrylic acid gives rise to molded SMC composites having the greatest tensile and impact strengths; (3) An optimum cure time and mold temperature exist for achieving the highest glass‐transition (Tg) of the low‐profile additive; (4) The values of cure time and mold temperature that have yielded the greatest tensile and impact strengths also yield molded specimens having the highest Tg of the low‐profile additive.