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Graphene‐Perovskite Fibre Photodetectors

Authors: S. Akhavan; A. Taheri Najafabadi; S. Mignuzzi; M. Abdi Jalebi; A. Ruocco; I. Paradisanos; O. Balci; +6 Authors

Graphene‐Perovskite Fibre Photodetectors

Abstract

AbstractThe integration of optoelectronic devices, such as transistors and photodetectors (PDs), into wearables and textiles is of great interest for applications such as healthcare and physiological monitoring. These require flexible/wearable systems adaptable to body motions, thus materials conformable to non‐planar surfaces, and able to maintain performance under mechanical distortions. Here, fibre PDs are prepared by combining rolled graphene layers and photoactive perovskites. Conductive fibres (~500 Ωcm‐1) are made by rolling single‐layer graphene (SLG) around silica fibres, followed by deposition of a dielectric layer (Al2O3 and parylene C), another rolled SLG as a channel, and perovskite as photoactive component. The resulting gate‐tunable PD has a response time~9ms, with an external responsivity~22kAW‐1 at 488nm for a 1V bias. The external responsivity is two orders of magnitude higher, and the response time one order of magnitude faster, than state‐of‐the‐art wearable fibre‐based PDs. Under bending at 4mm radius, up to~80% photocurrent is maintained. Washability tests show~72% of initial photocurrent after 30 cycles, promising for wearable applications.

Country
United Kingdom
Keywords

fibres, Condensed Matter - Materials Science, wearables, Condensed Matter - Mesoscale and Nanoscale Physics, graphene, Mesoscale and Nanoscale Physics (cond-mat.mes-hall), perovskites, photodetectors, Materials Science (cond-mat.mtrl-sci), FOS: Physical sciences, Physics - Applied Physics, Applied Physics (physics.app-ph)

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    Top 10%
    influence
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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
23
Top 10%
Average
Top 10%
Green
hybrid