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Advanced Optical Materials
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Exciton Collimation, Focusing and Trapping Using Complex Transition Metal Dichalcogenide Lateral Heterojunctions

Authors: Lamsaadi, Hassan; Cuche, Aurelien; Agez, Gonzague; Paradisanos, Ioannis; Beret, Dorian; Lombez, Laurent; Renucci, Pierre; +11 Authors

Exciton Collimation, Focusing and Trapping Using Complex Transition Metal Dichalcogenide Lateral Heterojunctions

Abstract

Abstract Controlling the motion of neutral excitons in optically active media is a mandatory development to enable the conception of advanced circuits and devices for applications in excitronics, quantum photonics, and optoelectronics. Recently, proof of unidirectional exciton transport from high‐ to low‐bandgap material is evidenced using a high‐quality lateral heterostructure separating transition metal dichalcogenide monolayers (TMD‐MLs). In this paper, by combining room‐temperature micro‐photoluminescence far‐field imaging with a statistical description of exciton transport, the underlying excitonic local distribution and fluxes taking place near lateral heterojunctions are unveiled. The complex 2D excitonic transport properties found near a linear interface separating WSe 2 from MoSe 2 TMD‐MLs are studied and reveal two distinct diffusion regimes profoundly affecting the effective diffusion length. Then, it is shown that combining two and three of these interfaces, allows advanced in‐plane control of the excitonic distribution and flux over large distances. Exciton focalization and trapping, allowing an increase in the local exciton density up to three orders of magnitude are demonstrated. Finally, flux collimation is achieved with the formation of parallel current lines extending a few micrometers away from the source. We believe that the deterministic shaping and positioning of the exciton distribution and flux shown here will be key toward the conception of realistic excitronic devices.

Country
France
Keywords

exciton flux, exciton diffusion exciton transfer exciton control exciton flux exciton kapitza resistance excitronics lateral heterostructure transition metal dichalcogenide, excitronics, lateral heterostructure, exciton transfer, transition metal dichalcogenide, [PHYS] Physics [physics], exciton kapitza resistance, exciton diffusion, exciton control

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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
3
Top 10%
Average
Average
Green
hybrid