A Long-term Gap-free High-resolution Air Pollutants concentration dataset (abbreviated as LGHAP) is of great significance for environmental management and earth system science analysis. In the current release of LGHAP aerosol dataset (LGHAP.v1), we provide a 21-year-long (2000–2020) gap free PM10 concentration product with daily 1-km resolution covering the land area of China. The dataset was generated from the daily gap free AOD (https://doi.org/10.5281/zenodo.5652257) that was derived through an integration of a set of data tensors of AOD and other related datasets such as air pollutants concentration and atmospheric visibility acquired from diversified sensors or platforms via a machine learned regression model. The dataset was provided in the NetCDF format, while data in each individual year were archived in a zip file. Python, Matlab, R, and IDL codes were also provided to help users read and visualize the LGHAP data.