Here we present semi-continuous and real-time measurements of elemental composition for PM2.5 and PM10 aerosols in Delhi, India, at a time resolution of 30 min to 1 h during two consecutive winters in 2018 and 2019, to identify the prevailing sources. Nine different aerosol sources were identified during both winters using positive matrix factorization (PMF), including dust, brake wear, a S-rich factor, two solid fuel combustion (SFC) factors and four industrial/combustion factors related to plume events (Cr-30 Ni-Mn, Cu-Cd-Pb, Pb-Sn-Se and Cl-Br-Se). Most of these sources had the highest relative contributions during late night (22:00 local time (LT)) and early morning hours (between 03:00 to 08:00 LT), which is consistent with enhanced emissions into a shallow boundary layer. Modelling of airmass source geography revealed that the pollutants enter Delhi via three distinct air corridors during winters including Nepal and Uttar Pradesh (India) in the east, and Pakistan, Punjab (India) and Haryana (India) in the north-west, during winter, when the national capital’s air quality is at its worst. This repository has excel file corresponding to each figures presented in main text published version.