The development of the IoT demands small, durable, remote sensing systems that have energy harvesters and storage. Various energy harvesters are developed, including piezoelectric, triboelectric, electromagnetic, and reverse-electrowetting-on-dielectric. However, integrating energy storage and sensing functionality receives little attention. This paper presents an electrochemical vibration sensor with a galvanic cell (Zn-Cu cell) as energy storage and a vibration transducer. The frequency response, scale factor, long-term response, impedance study, and discharge characteristics are given. This study proved the possibility of integrating energy storage and vibration sensing functionality with promising performance. The performance of the sensor halved within 74 min. The longevity of the sensor is short due to the spontaneous reactions and ions drained. The sensitivity can be restored after refilling the electrolyte. The sensor could be rechargeable by changing to a reversible electrochemical system such as a lead–acid cell in the future.