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Physical Review Letters
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Physical Review Letters
Article . 2000 . Peer-reviewed
License: APS Licenses for Journal Article Re-use
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Physical Review Letters
Article . 2001
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https://dx.doi.org/10.1103/phy...
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Sum-Frequency Vibrational Spectroscopy on Chiral Liquids: A Novel Technique to Probe Molecular Chirality

descriptionPublicationkeyboard_double_arrow_right Article 20 Nov 2000 English Publisher:American Physical Society (APS)Journal:Physical Review Letters, volume 85, pages 4,474-4,477 (issn: 0031-9007, eissn: 1079-7114, Copyright policy )
Authors: M A, Belkin; T A, Kulakov; K H, Ernst; L, Yan; Y R, Shen;

doi: 10.1103/physrevlett.85.4474

pmid: 11082574

Sum-Frequency Vibrational Spectroscopy on Chiral Liquids: A Novel Technique to Probe Molecular Chirality

Abstract

Optical activity in sum-frequency vibrational spectra has been observed for the first time in chiral liquids. The electric-dipole allowed chiral element of the nonlinear susceptibility appears to be 3 orders of magnitude smaller than typical allowed achiral elements. This is partly because the observed chirality requires a breakdown of the Born-Oppenheimer approximation.

Related Organizations
Keywords

Terpenes, Spectrum Analysis, Cyclohexenes, Molecular Conformation, Solvents, Stereoisomerism, Algorithms, Limonene

  • BIP!
    Impact byBIP!
    selected citations
    These citations are derived from selected sources.
    This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
    		 189
    popularity
    This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
    		 Top 10%
    influence
    This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
    		 Top 1%
    impulse
    This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
    		 Top 10%
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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
189
Top 10%
Top 1%
Top 10%
bronze