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Chemically vapor deposited Eu 3+ :Y 2 O 3 thin films as a material platform for quantum technologies

Nao Harada; Alban Ferrier; Diana Serrano; Mauro Persechino; Emrick Briand; Romain Bachelet; Ian Vickridge; +3 Authors

Chemically vapor deposited Eu 3+ :Y 2 O 3 thin films as a material platform for quantum technologies

Abstract

International audience; Rare earth ions hosted in solids are good candidates for quantum technologies due to their chemical stability and optical and spin transitions exhibiting long coherence lifetimes. While bulk oxide crystals are usually the preferred host material, the development of a scalable silicon-compatible thin film platform would be desirable. In this paper, we report on the growth of Y2(1-x)Eu2xO3 thin films on silicon in the full range of Eu3+ concentration by direct liquid injection Chemical Vapour Deposition. Our sub-micron polycrystalline films with a strong-(111) texture were grown for all compositions into the bixbyite cubic phase. The variation of growth rates with temperature and flow indicated that deposition occurred through a mass-transport controlled regime. Optical assessment of the Eu-doped thin films showed inhomogeneous linewidths as narrow as 50 GHz and fluorescence lifetimes of 1ms for the lowest concentrations. Finally, a spectral hole was successfully burned in a 200 nm-thin film with a 2 % Eu doping leading to a homogeneous linewidth of 11 MHz. These values are still below those reported for bulk single crystals indicating that additional decoherence mechanisms exist in such nanometric films, which might be alleviated by further improvement of the crystalline quality. Nevertheless, these results pave the way to the use of CVD-grown Eu:Y2O3 thin films as a platform for integrated quantum devices.

Country
France
Subjects by Vocabulary

ACM Computing Classification System: ComputingMilieux_MISCELLANEOUS

Microsoft Academic Graph classification: Optoelectronics business.industry business Crystallite Chemical vapor deposition Thin film Laser linewidth Doping Materials science Bixbyite Oxide chemistry.chemical_compound chemistry Silicon chemistry.chemical_element

Keywords

[PHYS.COND.CM-MS]Physics [physics]/Condensed Matter [cond-mat]/Materials Science [cond-mat.mtrl-sci], [PHYS.PHYS.PHYS-CHEM-PH]Physics [physics]/Physics [physics]/Chemical Physics [physics.chem-ph], [PHYS.QPHY]Physics [physics]/Quantum Physics [quant-ph], [PHYS.COND.CM-MS] Physics [physics]/Condensed Matter [cond-mat]/Materials Science [cond-mat.mtrl-sci], [PHYS.PHYS.PHYS-CHEM-PH] Physics [physics]/Physics [physics]/Chemical Physics [physics.chem-ph], [PHYS.QPHY] Physics [physics]/Quantum Physics [quant-ph], General Physics and Astronomy

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    Average
  • citations
    This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
    4
    popularity
    This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
    Average
    influence
    This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
    Average
    impulse
    This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
    Average
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citations
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
4
Average
Average
Average
Metrics badge
Funded by
EC| SQUARE
Project
SQUARE
Scalable Rare Earth Ion Quantum Computing Nodes
  • Funder: European Commission (EC)
  • Project Code: 820391
  • Funding stream: H2020 | RIA
Validated by funder
,
EC| NanOQTech
Project
NanOQTech
Nanoscale Systems for Optical Quantum Technologies
  • Funder: European Commission (EC)
  • Project Code: 712721
  • Funding stream: H2020 | RIA
Validated by funder | iis
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