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The Journal of Chemical Physics
Article . 2004 . Peer-reviewed
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Local-field effects on the spontaneous emission rate of CdTe and CdSe quantum dots in dielectric media

Authors: Wuister, S.F.; de Mello Donega, C.; Meijerink, A.;

Local-field effects on the spontaneous emission rate of CdTe and CdSe quantum dots in dielectric media

Abstract

The refractive index dependence of the spontaneous emission rate is determined using organically capped CdSe and CdTe quantum dots as probes. The radiative lifetime of the exciton emission is measured in a variety of apolar solvents with refractive indices n between 1.37 and 1.50. It is demonstrated that quantum dots provide a model system for testing theories on the influence of local-field effects on the spontaneous emission rate. The experimentally observed influence of n on the radiative lifetime is smaller than predicted by well-known models for local-field corrections but is in good agreement with a recently developed fully microscopic model for the local-field enhancement of the spontaneous emission rate.

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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
123
Top 10%
Top 10%
Top 10%
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