Precise Control of Molecular Dynamics with a Femtosecond Frequency Comb - A Weak Field Route to Strong Field Coherent Control

Preprint English OPEN
Pe'er, Avi ; Shapiro, Evgeny A. ; Stowe, Matthew C. ; Shapiro, Moshe ; Ye, Jun (2006)
  • Related identifiers: doi: 10.1103/PhysRevLett.98.113004
  • Subject: Physics - Optics | Physics - Atomic Physics | Physics - Atomic and Molecular Clusters | Quantum Physics

We present a general and highly efficient scheme for performing narrow-band Raman transitions between molecular vibrational levels using a coherent train of weak pump-dump pairs of shaped ultrashort pulses. The use of weak pulses permits an analytic description within t... View more
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