Precise Control of Molecular Dynamics with a Femtosecond Frequency Comb - A Weak Field Route to Strong Field Coherent Control

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Pe'er, Avi; Shapiro, Evgeny A.; Stowe, Matthew C.; Shapiro, Moshe; Ye, Jun; (2006)

We present a general and highly efficient scheme for performing narrow-band Raman transitions between molecular vibrational levels using a coherent train of weak pump-dump pairs of shaped ultrashort pulses. The use of weak pulses permits an analytic description within t... View more
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