Precise Control of Molecular Dynamics with a Femtosecond Frequency Comb - A Weak Field Route to Strong Field Coherent Control
Shapiro, Evgeny A.
Stowe, Matthew C.
Physics - Optics | Physics - Atomic Physics | Physics - Atomic and Molecular Clusters | Quantum Physics
We present a general and highly efficient scheme for performing narrow-band Raman transitions between molecular vibrational levels using a coherent train of weak pump-dump pairs of shaped ultrashort pulses. The use of weak pulses permits an analytic description within t...