publication . Preprint . 2006

Precise Control of Molecular Dynamics with a Femtosecond Frequency Comb - A Weak Field Route to Strong Field Coherent Control

Pe'er, Avi; Shapiro, Evgeny A.; Stowe, Matthew C.; Shapiro, Moshe; Ye, Jun;
Open Access English
  • Published: 01 Sep 2006
Abstract
We present a general and highly efficient scheme for performing narrow-band Raman transitions between molecular vibrational levels using a coherent train of weak pump-dump pairs of shaped ultrashort pulses. The use of weak pulses permits an analytic description within the framework of coherent control in the perturbative regime, while coherent accumulation of many pulse pairs enables near unity transfer efficiency with a high spectral selectivity, thus forming a powerful combination of pump-dump control schemes and the precision of the frequency comb. The concept is presented analytically and its feasibility and robustness are verified by simulations of dynamics...
Subjects
free text keywords: Quantum Physics, Physics - Atomic and Molecular Clusters, Physics - Atomic Physics, Physics - Optics
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[1] Th. Udem, R. Holzworth, and T. W. Hansch, Nature 416, 233 (2002); J. Ye, H. Schnatz, and L. W. Hollberg, IEEE J. Sel. Top. Quant. 9, 1041 (2003). S. T. Cundiff and J. Ye, Rev. Mod. Phys. 75, 325 (2003).

[2] A. Marian et al, Science 306, 2063 (2004); M. C. Stowe, F. C. Cruz, and J. Ye, Phys. Rev. Lett 96, 153001 (2006).

[3] M. Shapiro and P. Brumer, J. Chem. Phys. 84, 4103 (1986); D. J. Tannor and S. A. Rice, J. Chem. Phys. 83, 5013 (1985); M. Shapiro and P. Brumer, Rep. Prog. Phys. 66, 859942 (2003).

[4] U. Gaubatz et al, J. Chem. Phys. 92, 5363 (1990); N. Dudovich et al, Phys. Rev. Lett. 94, 083002 (2005); K. F. Lee et al, Phys. Rev. Lett. 93, 233601 (2004).

[5] N. V. Vitanov et al, Adv. At. Mol. Opt. Phys. 46, 55 (2001).

[6] H. Rabitz et al, Science 288, 824 (2000).

[7] P. S. Julienne, E. Tiesinga, and T. Kohler, J. Mod. Opt. 51, 1787 (2004); C. A. Regal et al, Nature 424, 47 (2003); M. W. Zwierlein et al, Phys. Rev. Lett. 91, 250401 (2003); S. Jochim et al, Science 302, 2101 (2003); T. Bourdel et al, Phys. Rev. Lett. 93, 050401 (2003).

[8] J. M. Sage et al, Phys. Rev. Lett. 94, 203001 (2005); C. M. Dion et al, Phys. Rev. Lett 86, 2253 (2001).

[9] C. P. Koch, R. Kosloff, and F. Masnou-Seeuws, Phys. Rev. A 73, 043409 (2006); E. Luc-Koenig et al, Phys. Rev. A 70, 033414 (2004).

[10] P. D. Drummond et al, Phys. Rev. A 65, 063619 (2002); M. Mackie et al, Phys. Rev. A 63, 043415 (2001).

[11] P. M. Morse, Phys. Rev. 34, 57 (1929); A. Frank, A. L. Rivera, and K. B. Wolf, Phys. Rev. A 61, 054102 (2000).

[12] A. M. Weiner, Rev. Sci. Inst. 71, 1929 (2000).

[13] B. M. Garraway and K. Suominen, Rep. Prog. Phys. 58, 365 (1995).

[14] C. J. Bardeen, Q. Wang, and C. V. Shank, Phys. Rev. Lett 75, 3410 (1995); J. Cao, C. J. Bardeen, and K. R. Wilson, Phys. Rev. Lett 80, 1406 (1998); V. S. Malinovsky and J. L. Krause, Phys. Rev. A 63, 043415 (2001).

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