Advanced source apportionment of carbonaceous aerosols by coupling offline AMS and radiocarbon size-segregated measurements over a nearly 2-year period

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Vlachou , Athanasia ; Daellenbach , Kaspar ; Bozzetti , Carlo ; Chazeau , Benjamin ; Salazar , Gary ; Szidat , Soenke ; Jaffrezo , Jean-Luc ; Hueglin , Christoph ; Baltensperger , Urs ; Haddad , Imad El ; Prévôt , André , (2018)
  • Publisher: European Geosciences Union
  • Journal: Atmospheric Chemistry and Physics (issn: 1680-7316, eissn: 1680-7324)
  • Related identifiers: doi: 10.7892/boris.116501, doi: 10.5194/acp-18-6187-2018
  • Subject: Chemistry | [ SDU.OCEAN ] Sciences of the Universe [physics]/Ocean, Atmosphere | QD1-999 | [ SDE.ES ] Environmental Sciences/Environmental and Society | [SDE.MCG]Environmental Sciences/Global Changes | Physics | [SDE.ES]Environmental Sciences/Environmental and Society | [SDU.OCEAN]Sciences of the Universe [physics]/Ocean, Atmosphere | [ CHIM.ANAL ] Chemical Sciences/Analytical chemistry | QC1-999 | [ SDE.MCG ] Environmental Sciences/Global Changes | 540 Chemistry | [CHIM.ANAL]Chemical Sciences/Analytical chemistry

Carbonaceous aerosols are related to adverse human health effects. Therefore, identification of their sources and analysis of their chemical composition is important. The offline AMS (aerosol mass spectrometer) technique offers quantitative separation of organic ... View more
  • References (76)
    76 references, page 1 of 8

    Agrios, K., Salazar, G. A., Zhang, Y. L., Uglietti, C., Battaglia, M., Luginbühl, M., Ciobanu, V. G., Vonwiller, M., and Szidat, S.: Online coupling of pure O2 thermo-optical methods - 14C AMS for source apportionment of carbonaceous aerosols study, Nucl. Instrum. Meth. B., 361, 288-293,, 2015.

    Aiken, A. C., Decarlo, P. F., Kroll, J. H., Worsnop, D. R., Huffman, J. A., Docherty, K. S., Ulbrich, I. M., Mohr, C., Kimmel, J. R., Sueper, D., Sun, Y., Zhang, Q., Trimborn, A., Northway, M., Ziemann, P. J., Canagaratna, M. R., Onasch, Z. B., Alfarra, M. R., Prevot, A. S., Dommen, J., Duplissy, J., Metzger, A., Baltensperger, U., and Jimenez, J. L.: O = C and OM = OC ratios of primary, secondary, and ambient organic aerosols with high-resolution time-of-flight aerosol mass spectrometry, Environ. Sci. Technol., 42, 4478-4485,, 2008.

    Alfarra, M. R., Prévôt, A. S. H., Szidat, S., Sandradewi, J.,Weimer, S., Lanz, V. A., Schreiber, D., Mohr, M., and Baltensperger, U.: Identification of the mass spectral signature of organic aerosols from wood burning emissions, Environ. Sci. Technol., 41, 5770- 5777,, 2007.

    Allan, J. D., Jimenez, J. L., Williams, P. I., Alfarra, M. R., Bower, K. N., Jayne, J. T., Coe, H., and Worsnop, D. R.: Quantitative sampling using an Aerodyne aerosol mass spectrometer - 1. Techniques of data interpretation and error analysis, J. Geophys. Res.-Atmos., 108, 4090,, 2003.

    Beekmann, M., Prévôt, A. S. H., Drewnick, F., Sciare, J., Pandis, S. N., Denier van der Gon, H. A. C., Crippa, M., Freutel, F., Poulain, L., Ghersi, V., Rodriguez, E., Beirle, S., Zotter, P., von der Weiden-Reinmüller, S. L., Bressi, M., Fountoukis, C., Petetin, H., Szidat, S., Schneider, J., Rosso, A., El Haddad, I., Megaritis, A., Zhang, Q. J., Michoud, V., Slowik, J. G., Moukhtar, S., Kolmonen, P., Stohl, A., Eckhardt, S., Borbon, A., Gros, V., Marchand, N., Jaffrezo, J. L., Schwarzenboeck, A., Colomb, A., Wiedensohler, A., Borrmann, S., Lawrence, M., Baklanov, A., and Baltensperger, U.: In situ, satellite measurement and model evidence on the dominant regional contribution to fine particulate matter levels in the Paris megacity, Atmos. Chem. Phys., 15, 9577-9591,, 2015.

    Bonvalot, L., Tuna, T., Fagault, Y., Jaffrezo, J. L., Jacob, V., Chevrier, F., and Bard, E.: Estimating contributions from biomass burning and fossil fuel combustion by means of radiocarbon analysis of carbonaceous aerosols: application to the Valley of Chamonix, Atmos. Chem. Phys., 16, 13753-13772,, 2016.

    Bozzetti, C., Daellenbach, K., R., Hueglin, C., Fermo, P., Sciare, J., Kasper-Giebl, A., Mazar, Y., Abbaszade, G., El Kazzi, M., Gonzalez, R., Shuster Meiseles, T., Flasch, M., Wolf, R., Krˇepelová, A., Canonaco, F., Schnelle-Kreis, J., Slowik, J. G., Zimmermann, R., Rudich, Y., Baltensperger, U., El Haddad, I., and Prévôt, A. S. H.: Size-resolved identification, characterization, and quantification of primary biological organic aerosol at a European rural site, Environ. Sci. Technol., 50, 3425-3434,, 2016.

    Bozzetti, C., Sosedova, Y., Xiao, M., Daellenbach, K. R., Ulevicius, V., Dudoitis, V., Mordas, G., Bycˇenkiene˙, S., Plauškaite˙, K., Vlachou, A., Golly, B., Chazeau, B., Besombes, J.-L., Baltensperger, U., Jaffrezo, J.-L., Slowik, J. G., El Haddad, I., and Prévôt, A. S. H.: Argon offline-AMS source apportionment of organic aerosol over yearly cycles for an urban, rural, and marine site in northern Europe, Atmos. Chem. Phys., 17, 117-141,, 2017a.

    Bozzetti, C., El Haddad, I., Salameh, D., Daellenbach, K. R., Fermo, P., Gonzalez, R., Minguillón, M. C., Iinuma, Y., Poulain, L., Elser, M., Müller, E., Slowik, J. G., Jaffrezo, J.-L., Baltensperger, U., Marchand, N., and Prévôt, A. S. H.: Organic aerosol source apportionment by offline-AMS over a full year in Marseille, Atmos. Chem. Phys., 17, 8247-8268,, 2017b.

    Bruns E., Krapf, M., Orasche, J., Huang, Y., Zimmermann, R., Drinovec, L., Mocˇnik, G., El-Haddad, I., Slowik, J. G., Dommen, J., Baltensperger, U., and Prévôt, A. S. H.: Characterization of primary and secondary wood combustion products generated under different burner loads, Atmos., Chem., Phys., 15, 2825-2841,, 2015.

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