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In-situ constraints on the vertical distribution of global aerosol

Authors: Watson-Parris, Duncan; Schutgens, Nick; Reddington, Carly; Pringle, Kirsty J.; Liu, Dantong; Allan, James D.; Coe, Hugh; +2 Authors

In-situ constraints on the vertical distribution of global aerosol

Abstract

Despite ongoing efforts, the vertical distribution of aerosols globally is poorly understood. This in turn leads to large uncertainties in the contributions of the direct and indirect aerosol forcing on climate. Using the Global Aerosol Synthesis and Science Project (GASSP) database – the largest synthesised collection of in-situ aircraft measurements currently available, with more than 1000 flights from 37 campaigns from around the world – we investigate the vertical structure of sub-micron aerosols across a wide range of regions and environments. The application of this unique dataset to assess the vertical distributions of number size distribution and Cloud Condensation Nuclei (CCN) in the global aerosol-climate model ECHAM-HAM reveals that the model underestimates accumulation mode particles in the upper troposphere, especially in remote regions. The processes underlying this discrepancy are explored using different aerosol microphysical schemes and a process sensitivity analysis. These show that the biases are predominantly related to aerosol ageing and removal rather than emissions.

116 references, page 1 of 12

Andrews, S. J., Jones, C. E., and Carpenter, L. J.: Aircraft measurements of very short-lived halocarbons over the tropical Atlantic Ocean, Geophys. Res. Lett., 40, 1005-01010, https://doi.org/10.1002/grl.50141, 2013.

Asa-Awuku, A., Moore, R. H., Nenes, A., Bahreini, R., Holloway, J. S., Brock, C. A., Middlebrook, A. M., Ryerson, T. B., Jimenez, J. L., DeCarlo, P. F., Hecobian, A., Weber, R. J., Stickel, R., Tanner, D. J., and Huey, L. G.: Airborne cloud condensation nuclei measurements during the 2006 Texas Air Quality Study, J. Geophys. Res.-Atmos., (1984-2012), 116, D11201, https://doi.org/10.1029/2010jd014874, 2011.

Barth, M. C., Cantrell, C. A., Brune, W. H., Rutledge, S. A., Crawford, J. H., Huntrieser, H., Carey, L. D., MacGorman, D., Weisman, M., Pickering, K. E., Bruning, E., Anderson, B., Apel, E., Biggerstaff, M., Campos, T., Campuzano-Jost, P., Cohen, R., Crounse, J., Day, D. A., Diskin, G., Flocke, F., Fried, A., Garland, C., Heikes, B., Honomichl, S., Hornbrook, R., Huey, L. G., Jimenez, J. L., Lang, T., Lichtenstern, M., Mikoviny, T., Nault, B., O'Sullivan, D., Pan, L. L., Peischl, J., Pollack, I., Richter, D., Riemer, D., Ryerson, T., Schlager, H., Clair, J. S., Walega, J., Weibring, P., Weinheimer, A., Wennberg, P., Wisthaler, A., Wooldridge, P. J., and Ziegler, C.: The Deep Convective Clouds and Chemistry (DC3) Field Campaign, B. Am. Meteorol. Soc., 96, 12810-1309, https://doi.org/10.1175/bamsd-13-00290.1, 2015.

Bergman, T., Kerminen, V.-M., Korhonen, H., Lehtinen, K. J., Makkonen, R., Arola, A., Mielonen, T., Romakkaniemi, S., Kulmala, M., and Kokkola, H.: Evaluation of the sectional aerosol microphysics module SALSA implementation in ECHAM5- HAM aerosol-climate model, Geosci. Model Dev., 5, 845-868, https://doi.org/10.5194/gmd-5-845-2012, 2012.

Berkoff, T. A., Welton, E. J., Campbell, J. R., Valencia, S., Spinhirne, J. D., Tsay, S.-C., and Holben, B. N.: Observations of Aerosols using the Micro-Pulse Lidar NETwork (MPLNET), IGARSS 2004. 2004 IEEE Int. Geosci. Remote Sens. Symp., 3, 2208-2211, https://doi.org/10.1109/igarss.2004.1370799, 2004.

Bezantakos, S., Barmpounis, K., Giamarelou, M., Bossioli, E., Tombrou, M., Mihalopoulos, N., Eleftheriadis, K., Kalogiros, J., D. Allan, J., Bacak, A., Percival, C. J., Coe, H., and Biskos, G.: Chemical composition and hygroscopic properties of aerosol particles over the Aegean Sea, Atmos. Chem. Phys., 13, 11595- 11608, https://doi.org/10.5194/acp-13-11595-2013, 2013. [OpenAIRE]

Brock, C. A., Cozic, J., Bahreini, R., Froyd, K. D., Middlebrook, A. M., McComiskey, A., Brioude, J., Cooper, O. R., Stohl, A., Aikin, K. C., de Gouw, J. A., Fahey, D. W., Ferrare, R. A., Gao, R.-S., Gore, W., Holloway, J. S., Hübler, G., Jefferson, A., Lack, D. A., Lance, S., Moore, R. H., Murphy, D. M., Nenes, A., Novelli, P. C., Nowak, J. B., Ogren, J. A., Peischl, J., Pierce, R. B., Pilewskie, P., Quinn, P. K., Ryerson, T. B., Schmidt, K. S., Schwarz, J. P., Sodemann, H., Spackman, J. R., Stark, H., Thomson, D. S., Thornberry, T., Veres, P., Watts, L. A., Warneke, C., and Wollny, A. G.: Characteristics, sources, and transport of aerosols measured in spring 2008 during the aerosol, radiation, and cloud processes affecting Arctic Climate (ARCPAC) Project, Atmos. Chem. Phys., 11, 2423- 2453, https://doi.org/10.5194/acp-11-2423-2011, 2011.

Canagaratna, M. R., Jayne, J. T., Jimenez, J. L., Allan, J. D., Alfarra, M. R., Zhang, Q., Onasch, T. B., Drewnick, F., Coe, H., Middlebrook, A., Delia, A., Williams, L. R., Trimborn, A. M., Northway, M. J., DeCarlo, P. F., Kolb, C. E., Davidovits, P., and Worsnop, D. R.: Chemical and microphysical characterization of ambient aerosols with the aerodyne aerosol mass spectrometer, Mass Spectrom. Rev., 26, 185-222, https://doi.org/10.1002/mas.20115, 2007.

Clarke, A. D.: A thermo-optic technique for in situ analysis of sizeresolved aerosol physicochemistry, Atmos. Environ. Part A, 25, 635-644, https://doi.org/10.1016/0960-1686(91)90061-B, 1991.

Clarke, A. D. and Kapustin, V. N.: A Pacific Aerosol Survey. Part I: A Decade of Data on Particle Production, Transport, Evolution, and Mixing in the Troposphere*, J. Atmos. Sci., 59, 363-382, https://doi.org/10.1175/1520- 0469(2002)059<0363:apaspi>2.0.co;2, 2002.

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citations
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
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